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Titlebook: Dissipative Exciton Dynamics in Light-Harvesting Complexes; Marco Schr?ter Book 2015 Springer Fachmedien Wiesbaden 2015 Molecular Physics.

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發(fā)表于 2025-3-21 20:01:31 | 只看該作者 |倒序?yàn)g覽 |閱讀模式
書(shū)目名稱Dissipative Exciton Dynamics in Light-Harvesting Complexes
編輯Marco Schr?ter
視頻videohttp://file.papertrans.cn/282/281637/281637.mp4
概述Includes supplementary material:
叢書(shū)名稱BestMasters
圖書(shū)封面Titlebook: Dissipative Exciton Dynamics in Light-Harvesting Complexes;  Marco Schr?ter Book 2015 Springer Fachmedien Wiesbaden 2015 Molecular Physics.
描述Marco Schr?ter investigates the influence of the local environment on the exciton dynamics within molecular aggregates, which build, e.g., the light-harvesting complexes of plants, bacteria or algae by means of the hierarchy equations of motion (HEOM) method. He addresses the following questions in detail: How can coherent oscillations within a system of coupled molecules be interpreted? What are the changes in the quantum dynamics of the system for increasing coupling strength between electronic and nuclear degrees of freedom? To what extent does decoherence govern the energy transfer properties of molecular aggregates?.
出版日期Book 2015
關(guān)鍵詞Molecular Physics; Molekülphysik; Photosynthese; Photosyntheses; Quantendynamik; Quantum Dynamics
版次1
doihttps://doi.org/10.1007/978-3-658-09282-5
isbn_softcover978-3-658-09281-8
isbn_ebook978-3-658-09282-5Series ISSN 2625-3577 Series E-ISSN 2625-3615
issn_series 2625-3577
copyrightSpringer Fachmedien Wiesbaden 2015
The information of publication is updating

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發(fā)表于 2025-3-21 21:36:32 | 只看該作者
Dissipative quantum dynamics,embedded in a protein environment. Within a quantum mechanical treatment it is practically impossible to take all degrees of freedom (DOFs) of such large systems explicitly into account. Note that there exist highly efficient methods, e.g., the multiconfiguration time-dependent Hartree method (MCTDH
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發(fā)表于 2025-3-22 00:28:57 | 只看該作者
Energy transfer in light-harvesting complexes,ibed via rate equations. Further, it was assumed that the structure of the photosynthetic units is optimized to maximize the quantum yield of the overall process. However, this simplified approach was questioned after the observation of long lasting coherent oscillations in the 2D-spectra of the FMO
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Dissipative quantum dynamics,rge systems explicitly into account. Note that there exist highly efficient methods, e.g., the multiconfiguration time-dependent Hartree method (MCTDH) [38], to treat the quantum dynamics of isolated systems, e.g., the intra-molecular dynamics of the aforementioned pigment molecules.
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Book 2015detail: How can coherent oscillations within a system of coupled molecules be interpreted? What are the changes in the quantum dynamics of the system for increasing coupling strength between electronic and nuclear degrees of freedom? To what extent does decoherence govern the energy transfer properties of molecular aggregates?.
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